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Polygodial: a viable natural product scaffold for the rapid synthesis of novel polycyclic pyrrole and pyrrolidine derivatives

Citation

Rihak, KJ and Bissember, AC and Smith, JA, Polygodial: a viable natural product scaffold for the rapid synthesis of novel polycyclic pyrrole and pyrrolidine derivatives, Tetrahedron, 74, (12) pp. 1167-1174. ISSN 0040-4020 (2018) [Refereed Article]

Copyright Statement

Copyright 2017 Elsevier Ltd.

DOI: doi:10.1016/j.tet.2017.10.015

Abstract

The dialdehyde polygodial was utilised as a chiral scaffold for the unified synthesis of novel polycyclic pyrrole and pyrrolidine derivatives. Mechanistic insight into the reaction of primary amines with this dialdehyde was obtained. In addition, one of these polycyclic pyrroles was transformed further to prepare novel pentacyclic frameworks.

Item Details

Item Type:Refereed Article
Keywords:polygodial, pyrrole, natural products, chiral synthetic scaffolds, heterocycles
Research Division:Chemical Sciences
Research Group:Organic Chemistry
Research Field:Organic Chemical Synthesis
Objective Division:Expanding Knowledge
Objective Group:Expanding Knowledge
Objective Field:Expanding Knowledge in the Chemical Sciences
UTAS Author:Rihak, KJ (Mr Kieran Rihak)
UTAS Author:Bissember, AC (Dr Alex Bissember)
UTAS Author:Smith, JA (Associate Professor Jason Smith)
ID Code:124734
Year Published:2018
Web of Science® Times Cited:5
Deposited By:Chemistry
Deposited On:2018-03-06
Last Modified:2019-02-27
Downloads:0

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